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Структура, динаміка та оптичні властивості фулеренів і фулеритів C60, C70: Автореф. дис… д-ра фіз.-мат. наук / Ю.І. Прилуцький, Київ. ун-т ім. Т.Шев

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EE?ANUeEEE OI?AA?NEOAO ?iai? OA?ANA Oaa/aiea

I?EEOOeUeEEE TH??e ?aaiiae/

OAeE 538.9; 535.33; 532.73

NO?OEOO?A, AeEIAI?EA OA IIOE*I? AEANOEAINO?

OOEA?AI?A ? OOEA?EO?A N60, N70

01.04.02 – oai?aoe/ia o?ceea

AAOI?AOA?AO

aeena?oaoe?? ia caeiaoooy iaoeiaiai nooiaiy

aeieoi?a o?ceei-iaoaiaoe/ieo iaoe

EE?A – 1998

Aeena?oaoe??th ? ?oeiien.

?iaioa aeeiiaia a Ee?anueeiio oi?aa?neoao? ?iai? Oa?ana Oaa/aiea ia
eaoaae?? oai?aoe/ii? o?ceee.

Iaoeiaee eiinoeueoaio: aeieoip oiceei-iaoaiaoe/ieo iaoe, ipioanip
I?ieaae/ ?ai? Iaaeiae/, caa?aeoaa/ eaoaae?e oai?aoe/ii? o?ceee
Ee?anueeiai oi?aa?neoaoo ?iai? Oa?ana Oaa/aiea

Io?oe?ei? iiiiaioe:

aeieoi? o?ceei-iaoaiaoe/ieo iaoe Aaae??iei Aiaoie?e Aioiiiae/,
i?ia?aeiee iaoeiaee ni?a?ia?oiee O?ceei-oaoi?/iiai ?inoeoooo iecueeeo
oaiia?aoo? ?i. A.?. A??e?ia IAI Oe?a?ie (i. Oa?e?a)

aeieoi? o?ceei-iaoaiaoe/ieo iaoe, i?ioani? ?aaiia Ieoaeei Ieaen?eiae/,
caa?aeoaa/ a?aeae?eo oai??? ia?aeaaeueieo e?enoae?a ?inoeoooo
iaoaeio?ceee ?i. A.A. Eo?aethiiaa IAI Oe?a?ie (i. Ee?a)

aeieoi? o?ceei-iaoaiaoe/ieo iaoe Eoi???ae/ A?eoi? Aiaoie?eiae/,
i?ia?aeiee iaoeiaee ni?a?ia?oiee ?inoeoooo oai?aoe/ii? o?ceee ?i. I.I.
Aiaiethaiaa IAI Oe?a?ie (i. Ee?a)

I?ia?aeia onoaiiaa: ?inoeooo o?ceee eiiaeainiaaieo nenoai IAI Oe?a?ie
(i. Euea?a)

Caoeno a?aeaoaeaoueny 22 a?oaeiy 1998 ?. i 1430 aiae. ia can?aeaii?
niaoe?ae?ciaaii? a/aii? ?aaee Ae 26.001.08 i?e Ee?anueeiio oi?aa?neoao?
?iai? Oa?ana Oaa/aiea ca aae?anith: 252022 Ee?a, i?iniaeo aeaae.
Aeooeiaa, 6, o?ce/iee oaeoeueoao, aoae. 500.

C aeena?oaoe??th iiaeia iciaeiieoeny o a?ae?ioaoe? Ee?anueeiai
oi?aa?neoaoo ?iai? Oa?ana Oaa/aiea ca aae?anith: 252033, Ee?a,
aoe.Aieiaeeie?nueea 58.

Aaoi?aoa?ao ?ic?neaiee 10 eenoiiaaea 1998 ?.

A/aiee nae?aoa? niaoe?aaee

ae.o.-i.i., i?ioani? Iiia?aiei E.A.

CAAAEUeIA OA?AEOA?ENOEEA ?IAIOE

Aeooaeuei?noue oaie. C na?aaeeie 80-o ?ie?a ?icii/aoi ?ioaineaia
aeine?aeaeaiiy ooea?ai?a [1] – aaaaoiaoiiieo eeanoa??a aoaeaoeth Cn, aea
n – /enei aoii?a aoaeaoeth, ye? ciaoiaeyoueny ia caieioo?e (noa?e/i?e /e
noa?i?aeaeuei?e) iiaa?oi? iieaeoee, neiao?e/iei /eiii iie?eo?e
i?aaeeueieie i’yoeeooieeaie (?o anueiai 12) ? oanoeeooieeaie (ca
oai?aiith Aeea?a ?o iiaea aooe n/2 – 10). Na?aae iiaeeeaeo oei?a
ooea?ai?a iaea?eueo noaa?eueieie ? iieaeoee N60 ? N70 [2]. Neiao??y
ooea?aio N60 iieno?oueny a?oiith ?einaaae?a [1], yea aeiaaee /an ia
aeeeeeaea iniaeeaiai ?ioa?ano, ine?eueee ia aoee a?aeii? ?aaeuei?
o?ce/i? ia’?eoe, ui i?noyoue na?aae iiai?ioieo aeaiaio?a neiao??? a?nue
i’yoiai ii?yaeeo.

O 1991?. aoea ?ic?iaeaia oaoiieia?y iaea?aeaiiy ooea?ai?a o
iae?ineii?/i?e e?eueeino?, ui caniiaaia ia oa?i?/iiio ?icieeaii?
a?ao?oiaeo aeaeo?iae?a o aeoaiaiio ?ic?yae? [3]. Aiia a?aee?eea aeinooi
aei aea/aiiy ooea?ai?a ia o?eueee o iieaeoey?i?e oi?i?, aea oaeiae o
e?enoae?/iiio noai? (ooea?eo?).

Aeine?aeaeaiiy aeaeo?e/ieo ? iaai?oieo aeanoeainoae aeiiiaaieo eoaeieie
aeaiaioaie ooea?ai?a i?eaaei aei a?aee?eooy o 1991?. iaaei?ia?aeiino? o
eoaiaaieo ooea?eoao (ooea?eaeao) [4]. O oeueiio ae ?ioe? aoea aeyaeaia
ua iaeia oe?eaaa iniaeea?noue ooea?ai?a – caeaoi?noue ooai?thaaoe
o?oa/ao? aieieia (iaiio?oaee), ye? a?eueo no?ee? aei o?i?/ii? ae??,
oiio? ? i?oei?o? ca ?io? a?aeii? aieieia. A caeaaeiino? a?ae
aaiiao?e/ieo ia?aiao??a iaiio?oaea iiaea iaoe aeanoeaino? a?ae iaoaeo
aei ae?aeaeo?eea [5].

O 1995?. aoee neioaciaai? aaoa?iooea?aie (iieaeoee ooea?ai?a, o yeeo
iaeei /e aeae?eueea aoii?a aoaeaoeth cai?uai? aoiiaie ?ioiai ni?oo) oa
io?eiai? aiaei? ?ic/eie ooea?ai?a N60, N70 [6].

Ioaea, aeeiiai? a inoaii? ?iee aenia?eiaioaeuei? aeine?aeaeaiiy
o?ceei-o?i?/ieo aeanoeainoae ooea?ai?a aeacothoue ia oe?ie?, a ?ieiee
oi?eaeuei? ia?niaeoeae ?o i?aeoe/iiai aeei?enoaiiy, cie?aia, a
i?e?iaeaeo?ii?oe? (aaoa?iooea?aie ye iniiaa aeey iiaeo iaaei?ia?aeiee?a
oa oioiaeaeo?iiieo i?eeaae?a, aoaeaoeaa? iaiio?oaee ye ?cieyoe?eiee
iaoa??ae oa aaoa?ino?oeoo?e), iaaeeoeei? (ooea?aie ye ni?aaioe,
iaiio?oaea ye can?a o?ainii?ooaaiiy a ee?oeio e?eoaaeueieo i?aia?ao?a),
oaoi?oe? (ooea?eoe ye iniiaa aeey neioaco ooo/ieo aeiac?a, ooea?aie ye
aeii?oee aei ianoeeueieo ?a/iaei oa ?iii? aeiaethaa/? aeey aoii?a
?aae?iaeoeaieo aeaiaio?a, ?ic/eie ooea?ai?a ye iniiaa aeey noai?aiiy
iae?i?eieo iioe/ieo caoai??a) [4-5]. O ca’yceo c oeei aeieeea
iaiao?aei?noue oai?aoe/iiai iaa?oiooaaiiy io?eiaieo ?acoeueoao?a ? ia ?o
iniia? ia?aaeaa/aiiy iiaeo aoaeo?a. A ia?oo /a?ao oea noino?oueny
aeine?aeaeaiiy no?oeoo?e oa iaoai?/ieo aeanoeainoae ooea?ai?a ?
ooea?eo?a a caeaaeiino? a?ae oaiia?aoo?e oa ciai?oiueiai oeneo.
Iio?aaothoue aeaoaeueiiai aea/aiiy ?o eieeai? niaeo?e, ine?eueee aiie
iaiao?aei? aeey iiaoaeiae ei?aeoieo i?aeiieaeoey?ieo iioaioe?ae?a, ye?
aecia/athoue i?oaei? eiinoaioe oa oa?iiaeeiai?/i? ia?aiao?e oeeo nenoai.
E??i oiai, caeeoathoueny aeooaeueieie aeine?aeaeaiiy iaoai?ci?a
iaaei?iaiaeiinoi o ooea?eaeao N60 [4], ye? a?aoiaothoue iecueei/anoioii
(e?a?aoe?ei?) oiiiie oa aioo??oiueiiieaeoey?i? (yi-oaeea??anuee?)
eieeaaiiy. Iiaeeaeaii? oaaae caneoaiao? aea/aiiy no?oeoo?ieo
aeanoeainoae aiaeieo ?ic/ei?a ooea?ai?a, ine?eueee aiie ? i?ioioeiaie
iiaiai eeano iaaee/ieo i?iaeoeo?a [6]. Ia?aoo?, aeeeeea? cia/iee ?ioa?an
aeine?aeaeaiiy aeeiai?ee o?eieaoii caoaeaeaieo noai?a ooea?eo?a a
caeaaeiino? a?ae oaiia?aoo?e oa iaai?oiiai iiey [7-9], ine?eueee oe?
noaie a?ae?-a?athoue aaaeeeao ?ieue o aaaaoueio o?ce/ieo i?ioeanao
(oinoi?anoeaioe??, oiia?eueiai?e oethi?anoeaioe??,
aeaeo?iethi?i?noeaioe??, ia?aiino aia?a??, oioii?ia?aeiino?).

Ioaea, iaoith aeena?oaoe?eii? ?iaioe ? oai?aoe/ia aeine?aeaeaiiy
no?oeoo?ieo oa iioe/ieo aeanoeainoae iaea?eueo noaa?eueieo ooea?ai?a ?
ooea?eo?a N60, N70, a oaeiae aeeiai?ee o?eieaoii caoaeaeaieo noai?a o
oeeo iieaeoey?ieo nenoaiao a iaaeao cai?iiiiiaaieo ?ic?aooieiaeo
iiaeaeae.

O a?aeiia?aeiino? aei aeua cacia/aieo o?ce/ieo i?iaeai noi?ioeueiaai?
oae? iniiai? caaea/? aeine?aeaeaiiy:

( ?ic?aooiie yi-oaeea??anueeeo aeaoi?iaoe?e oa yi-oaeea??anueeeo
?icuaieaiue eieeaieo iiae iieaeoee N60;

( ?ic?aooiie ??aiiaaaeieo no?oeoo? ooea?eo?a N60 ? N70, niaeo??a ?o
i?aeiieaeoey?ieo eieeaaiue, oaeaeeinoae caoeo ? eiinoaio i?oaeiino?;

( ?ic?aooiie no?oeoo?e ooea?aiiaeo aa?aaao?a N60 o aiaeiiio ?ic/ei?;

( ?ic?aooiie eiia??iinoae ni?i-a?aoeiai? ?aeaenaoe?? o o?eieaoii
caoaeaeaieo noaiao ooea?eo?a N60 ? N70;

( ?ic?aooiie eiia??iinoae ia?aoiae?a o o?eieaoii caoaeaeaieo noaiao
ooea?eo?a N60 ? N70 i?ae ae??th aeonoe/ii? oaee?;

( ii??aiyiiy ?acoeueoao?a oai?aoe/ieo ?ic?aooie?a c iayaieie
aenia?eiaioaeueieie aaee/eiaie oa ia?aaeaa/aiiy iiaeo aoaeo?a.

Iaoeiaa iiaecia iaea?aeaieo ?acoeueoao?a. I?iaaaeai? aeine?aeaeaiiy
i?aeii?yaeeiaai? ?icaeoeo iiaiai iaoeiaiai iai?yieo o o?ceoe?
eiiaeainiaaiiai noaio – oai??? ooea?ai?a. O aeena?oaoe?ei?e ?iaio?
aia?oa:

1. I?iaaaeaiee e?euee?niee aiae?c aeeiai?/iiai aoaeoo ssia-Oaeea?a o
ooea?ai? N60, aeei?enoiaoth/e eieeaio iiaeaeue c i?i?iaeueiei /eneii
ia?aiao??a.

2. Aeine?aeaeaia iecueeioaiia?aoo?ia i???ioaoe?eii aii?yaeeiaaia
e?enoae?/ia oaca ooea?ai?a N60 ? N70 a caeaaeiino? a?ae ciai?oiueiai
oeneo. I?iaaaeaiee oai?aoeei-a?oiiaee aiae?c aeeiai?/ii? caaea/? aeey
ooea?eo?a N60 ? N70 o aeiaaioaeeueiaiio iaaeeaeaii?. ?ic?aoiaai?
cia/aiiy /anoio ? oi?ie i?aeiieaeoey?ieo eieeaaiue oeeo e?enoae?a a
oeaio?? ciie A??eethaia. Io?eiai? aiae?oe/i? ae?ace aeey ia/eneaiiy
oaeaeeinoae caoeo o ooea?eoao N60 ? N70 oa eiinoaio i?oaeiino? aeey
e?enoaea N70.

3. Aeine?aeaeaia no?oeoo?a ooea?aiiaeo aa?aaao?a N60 o aiaeiiio ?ic/ei?.

4. Aeine?aeaeai? iecueeioaiia?aoo?i? iaoai?cie ni?i-a?aoeiai?
?aeaenaoe?? o o?eieaoii caoaeaeaieo noaiao ooea?eo?a N60 ? N70, ye?
a?aoiaothoue:

– ca’ycie iinooiaeueieo ? iaa?oaeueieo ?oo?a iieaeoee;

– ca’ycie iinooiaeueieo ?oo?a iieaeoee ? aioo??oiueiiieaeoey?ieo
eieeaaiue ?? yaea?.

5. Io?eiaea iiaeaeueoee ?icaeoie oai??y aeonoioinoi?anoeaioiiai
iiaea?eiiai ?aci-iaino o aeii?oeiaeo iieaeoey?ieo e?enoaeao. Eiia??iino?
ia?aoiae?a o o?eieaoii caoaeaeaieo noaiao ooea?eo?a N60 ? N70 i?ae
ae??th aeonoe/ii? oaee? aeine?aeaeai? a caeaaeiino? a?ae iai?yieo ??
iioe?aiiy o oeeo e?enoaeao.

I?aeoe/ia cia/aiiy oa a??ia?aei?noue iaea?aeaieo ?acoeueoao?a.
I?iaaaeai? oai?aoe/i? aeine?aeaeaiiy iiyniththoue ?yae
aenia?eiaioaeueieo oaeo?a [10-13]:

( caeaaei?noue /anoio e?a?aoe?eieo eieeaaiue aeey ooea?eoo N60 a?ae
aaee/eie ciai?oiueiai oeneo;

( cia/aiiy aaee/eie iiaeoey ia’?iiiai noeneo aeey ooea?eoo N60;

( cia/aiiy aaee/ei eiinoaio i?oaeiino? aeey ooea?eoo N70;

( oaiia?aoo?io caeaaei?noue /ano ni?i-a?aoeiai? ?aeaenaoe?? o o?eieaoii
caoaeaeaieo noaiao ooea?eoo N60.

?ic?aoiaai? cia/aiiy /anoio aioo??oiueiiieaeoey?ieo eieeaaiue ooea?ai?a
N60 ? N70, no?oeoo?a oa niaeo? i?aeiieaeoey?ieo eieeaaiue ooea?eo?a N60
? N70 aeia?a ocaiaeaeothoueny c iayaieie aenia?eiaioaeueieie aaee/eiaie
[14-20].

A??ia?aei?noue io?eiaieo ?acoeueoao?a caaacia/o?oueny oaeiae
iaa?oioiaai?noth i?eeiyoeo oai?aoe/ieo iiaeaeae, oe?ieei canoinoaaiiyi
caaaeueieo i?eioeei?a neiao???, aeia?a ?icaeiaieo iaoiae?a oai??? a?oi
oa eaaioiai? iaoai?ee, aeei?enoaiiyi a?aeiia?aeiiai iaoaiaoe/iiai
aia?aoo a iaaeao /eneiaeo ?ic?aooie?a.

?acoeueoaoe aeena?oaoe?eii? ?iaioe iiaeooue oe?eeii aooe aeei?enoai?
aeey ii-aeaeueoiai aeine?aeaeaiiy iaoai?/ieo, iioe/ieo ? aeaeo?iiieo
aeanoeainoae aoaeaoeaaeo iaiio?oaie oa oiiiiieo iaoai?ci?a
iaaei?ia?aeiino? o ooea?eaeao.

Ia caoeno aeiinyoueny oae? iniiai? iieiaeaiiy:

1. ?acoeueoaoe ?ic?aooieo yi-oaeea??anueeeo aeaoi?iaoe?e oa ?icuaieaiue
aeoeaieo yi-oaeea??anueeeo iiae ooea?aio N60 a iaaeao eieeaii? iiaeae? c
i?i?iaeueiei /eneii ia?aiao??a (/ioe?e iacaeaaei? neeia? noae?).

2. Oai?aoeei-a?oiiaee aiae?c aeeiai?/ieo caaea/ aeey ooea?eo?a N60, N70,
ui aea? iiaeeea?noue ca aiae?oe/ieie oi?ioeaie ia/eneeoe cia/aiiy /anoio
? oi?ie i?ae- iieaeoey?ieo eieeaaiue oeeo e?enoae?a a oeaio?? ciie
A??eethaia, oaeaeeino? caoeo a ieo oa ?oi? eiinoaioe i?oaeiino?.

3. Iiaeaeueiee ?ic?aooiie iecueeioaiia?aoo?ieo ??aiiaaaeieo no?oeoo?
ooea?eo?a N60, N70 oa ?o eieeaieo niaeo??a a caeaaeiino? a?ae
ciai?oiueiai oeneo.

4. ?acoeueoaoe ?ic?aooieo no?oeoo?e ooea?aiiaeo aa?aaao?a N60 o aiaeiiio
?ic/ei?, ui ia?aaeaa/a? ?nioaaiiy o iueiio noaa?eueieo a?ae?aoiaaieo
eeanoa??a oa e?enoae?o?a.

5. Oai??y iecueeioaiia?aoo?ii? ni?i-a?aoeiai? ?aeaenaoe?? o o?eieaoii
caoaeaeaieo noaiao ooea?eo?a N60, N70, yea a?aoiao? ca’ycie
iinooiaeueieo ?oo?a iieaeoee c ?? iaa?oaeueieie ?ooaie oa
aioo??oiueiiieaeoey?ieie ci?uaiiyie yaea?.

Ca’ycie ?iaioe c iaoeiaeie i?ia?aiaie, ieaiaie, oaiaie. Aeena?oaoe?eia
?iaioa aeeiioaaeany a iaaeao iaoeiaiai i?iaeoo
“Oinoi?anoeaioii-i?e?ioaeeueiaee ?aciiain oa ni?i-naeaeoeaia aeeiai?ea
o?eieaoieo caoaeaeaiue a iieaeoey?ieo e?enoaeao o neeueieo iaai?oieo
iieyo i?e iecueeeo oaiia?aoo?ao” (Aea?aeaaia iaoeiai-oaoi?/ia i?ia?aia N
2/186 “O?eieao” a?ae 24.06.1992?.) oa o a?aeiia?aeiino? c ieaiii
iaoeiai-aeine?aeieoeueei? ?iaioe eaoaae?e oai?aoe/ii? o?ceee Ee?anueeiai
oi?aa?neoaoo ?iai? Oa?ana Oaa/aiea “O?ceei-iaoaiaoe/ia i?iaiicoaaiiy
iiaeo o?ce/ieo aeanoeainoae iaoa??ae?a, ia’?eo?a ? na?aaeiaeu,
iaoiiaeaieo ?o aca?iiae??th c aei?ii?ithaaiiyi, oa iaoanoaa?euei? oacia?
noaie ?a/iaeie” (Aea?aeathaeaeaoia oaia N 970 26 a?ae 01.01.1997?.).

Ai?iaaoe?y ?acoeueoao?a aeena?oaoe??. Iniiai? ?acoeueoaoe aeena?oaoe??
aeiiia?aeaeeny ? iioae?eiaai? a iaoa??aeao oaeeo iaoeiaeo eiioa?aioe?e:
I?aeia?iaeia eiioa?aioe?y c iaaiaoecio (Aa?oaaa, Iieueua, 1994?.);
?a?iiaenueea aeine?aeieoeueea eiioa?aioe?y c aeaeo?iiii? no?oeoo?e
oaa?aeeo o?e (Aaonaeae, Ii?aaa?y, 1994?.); 3 ? 4 I?aeia?iaei? oeiee c
neiao??? oa no?oeoo?ieo aeanoeainoae eiiaeainiaaiiai noaio (Iiciaiue,
Iieueua, 1994?.; Cay/eiai, Iieueua, 1996?.); 1 ? 2 I?aeia?iaei?
oeiee-eiioa?aioe?? “Aeaeo?iii? i?ioeane a i?aai?/ieo iaoa??aeao” (Ee?a,
1995?., 1998?.); 2 ? 3 I?aeia?iaei? oeiee “Ooea?aie ? aoiii? eeanoa?e”
(N.-Iaoa?ao?a, ?in?y, 1995?., 1997?.); XII ? XIII Iaoe?iiaeuei?
oeiee-nai?ia?e “Niaeo?ineii?y iieaeoe oa e?enoae?a” (I?aeei, 1995?.;
Noie, 1997?.); XXI I?aeia?iaeia eiioa?aioe?y c o?ceee iecueeeo
oaiia?aoo? (I?aaa, *ao?y, 1996?.); 10 Eiioa?aioe?y ?a?iiaenueeiai
o?ce/iiai oiaa?enoaa “Oaiaeaioe?? o o?ceoe?” (Naa?euey, ?niai?y,
1996?.); Eiioa?aioe?y c ab initio ?ic?aooie?a neeaaeieo i?ioean?a o
iaoa??aeao (Oaueia?o-Aithiae, I?ia//eia, 1996?.); Eiioa?aioe?y c
iecueeeo oaiia?aoo? (No?ana E?nia, Neiaa//eia, 1996?.); 32 Ceiiaa oeiea
c oai?aoe/ii? o?ceee (Ea?ia/, Iieueua, 1996?.); XII Eiioa?aioe?y c
oaa?aeiai o?ea (Caeiiaia, Iieueua, 1996?.); I?aeia?iaeia iaoeiaa
eiioa?aioe?y “Iaoaiaoe/i? iiaeae? iae?i?eieo caoaeaeaiue, ia?aiino,
aeeiai?ee, ea?oaaiiy a eiiaeainiaaieo nenoaiao oa ?ioeo na?aaeiaeuao”
(Oaa?, ?in?y, 1996?.); 15 oa 16 Caaaeuei? eiioa?aioe?? c o?ceee
eiiaeainiaaiiai noaio (No?ana-Aaaaia, ?oae?y, 1996?.; E?oa?i, Aaeuea?y,
1997?.); Nai?ia? e?a?i NIAe “Ooea?aie-97” (Ee?a, 1997?.); Aaniyia
can?aeaiiy ?a?iiaenueeiai oiaa?enoaa c aeine?aeaeaiiy iaoa??ae?a
(No?anao?a, O?aioe?y, 1997?., 1998?.); 5 I?aeia?iaeiee neiiic?oi c
aeine?aeaeaiue o neeueieo iaai?oieo iieyo (N?aeiae, Aano?ae?y, 1997?.);
5 I?aeia?iaeiee A?aia??anueeee neiiic?oi c oai??? a?oi (A?aeaiue,
Aano??y, 1997?.); ?a?iiaenueea eiioa?aioe?y c o?i?? oa o?ceee
aaaaoiooie- oe?iiaeueieo iaoa??ae?a (Ani?ioi, Ii?ooaae?y, 1997?.); 2
I?aeia?iaeia oeiea c aenieeo oaoiieia?e (N.-Iaoa?ao?a, ?in?y, 1998?.);
XXIV ?a?iiaenueeee eiia?an c iieaeoey?ii? niaeo?ineii?? (I?aaa, *ao?y,
1998?.); 5 I?aeia?iaeia eiioa?aioe?y c iaiioeaeueii? iaoee ? oaoiieia??
(A??i?iaai, Aiae?y, 1998?.); 9 I?aeia?iaeiee neiiic?oi c iaeeo /anoeiie
oa iai?aai?/ieo eeanoa??a (Eocaia, Oaaeoea??y, 1998?.); Eiioa?aioe?y c
eiii’thoa?ii? o?ceee (A?aiaaea, ?niai?y, 1998?.); I?aeia?iaeia
eiioa?aioe?y “O?ceea 21 noie?ooy” (N.-Iaoa?ao?a, ?in?y, 1998?.).

Io?eiai? ?acoeueoaoe aeiiia?aeaeeny ? iaaiai?thaaeeny ia nai?ia?ao
eaoaae?e oai?aoe/ii? o?ceee Ee?anueeiai oi?aa?neoaoo ?iai? Oa?ana
Oaa/aiea, ?inoeoooo oai?aoe/ii? o?ceee ?i. I.I. Aiaiethaiaa IAI Oe?a?ie
(Ee?a), ?inoeoooo iaoaei- o?ceee ?i. A.A. Eo?aethiiaa IAI Oe?a?ie
(Ee?a), ?inoeoooo yaea?ieo aeine?aeaeaiue IAI Oe?a?ie (Ee?a),
O?ceei-oaoi?/iiai ?inoeoooo iecueeeo oaiia?aoo? ?i. A.?. A??e?ia IAI
Oe?a?ie (Oa?e?a), ?inoeoooo o?ceee eiiaeainiaaieo nenoai IAI Oe?a?ie
(Euea?a), eaai?aoi??? c ian-niaeo?iiao??? ?inoeoooo oa?ai?? AII Oe?a?ie
(Oa?e?a), eaai?aoi??? c iaaei?ia?aeiino? oa iaaiaoecio Iieaeaanueeiai
aea?aeaaiiai oi?aa?neoaoo (Eeoei?a), ?inoeoooo oai?aoe/ii? o?ceee
A?ioeeaanueeiai oi?aa?neoaoo (Iieueua), a oaeiae ia iaoeiaeo nai?ia?ao
c? noaoenoe/ii? oai??? eiiaeainiaaieo nenoai o Euea?anueeiio
aea?aeaaiiio oi?aa?neoao? ?i. ?. O?aiea oa “Iae?i?ei? nenoaie oa ?o
iiaeae?” a Iineianueeiio aea?aeaaiiio oi?aa?neoao? ?i. I. Eiiiiiniaa
(?in?y).

Aei iniaenoiai aianeo caeiaoaa/a a iaea?aeaiiy iaoeiaeo ?acoeueoao?a
iaeaaeaoue:

– iinoaiiaea caaea/ aeine?aeaeaiiy;

– i?iaaaeaiiy on?o aiae?oe/ieo aeeeaaeie;

– i?iaaaeaiiy /eneiaeo ?ic?aooie?a ni?eueii c ni?aaaoi?aie a iaaeao
iiaeaeae, cai?iiiiiaaieo aaoi?ii;

– aiae?c oai?aoe/ieo ?acoeueoao?a ia iniia? ii??aiyiiy c iayaieie
aenia?e- iaioaeueieie aeaieie oa ia?aaeaa/aiiy iiaeo aoaeo?a.

Ioae?eaoe?? caeiaoaa/a. Ca iaoa??aeaie aeena?oaoe?? iioae?eiaaii 48
?ia?o: 21 noaooth o ?aoa?iaaieo iaoeiaeo aeo?iaeao, 4 noaoo? o
?aoa?iaaieo ca??ieeao iaoeiaeo i?aoeue oa 23 oace o iaoa??aeao iaoeiaeo
eiioa?aioe?e. Iniiai? ?acoeueoaoe aeena?oaoe?? i?aaenoaaeai? o 18
i?aoeyo, a oiio /ene? 10 iaeiiin?aieo. ?o ia?ae?e iiaeaii a e?ioe?
aaoi?aoa?aoo.

O ?iaioao [1A, 3A, 5A-8A, 13A], aeeiiaieo o ni?aaaoi?noa?, aeena?oaioo
iaeaaeaoue iinoaiiaea caaea/ aeine?aeaeaiiy, ?ic?iaea oa aea?? iaoiae?a
?o ?ica’ycaiiy, aiae?c oa ?ioa?i?aoaoe?y io?eiaieo ?acoeueoao?a,
iaienaiiy oaenoo noaoae. *eneia? ?ic?aooiee aeeiiai? ni?eueii c
Oaiiaaeiaei A.A., Aeo?iaei N.N. oa Iaca?aieii I.A. [1A, 5A, 8A, 13A,
18A]. Ni?aaaoi?e Aiae?a?a A.I. [1A, 3A, 5A-7A] oa Aoaaiia A.I. [13A]
a?aee o/anoue a iaaiai?aii? io?eiaieo ?acoeueoao?a. Aenia?eiaioaeueia
/anoeia ?iaioe [18A] aeeiiaia ni?aaaoi?aie Aocaiueiaith ?.A., Aoeaa?iei
E.A., Iiai??eiaei A.?., ssuoeii A.I., Anoaoe?iei TH.A., Iaoeue/ainueeei
O.TH., Aiae???anueeei A.A. oa Oa?oii I.

No?oeoo?a oa ia’?i aeena?oaoe??. Aeena?oaoe?y neeaaea?oueny ?c anooio,
/ioe?ueio ?icae?e?a, aeniiae?a, aeaio aeiaeaoe?a ? nieneo aeei?enoaieo
aeaea?ae. ?iaioa aeeeaaeaia ia 163 noi??ieao ae?oeiaaiiai oaenoo ?
i?noeoue 17 oaaeeoeue oa 25 ?enoie?a. Nienie ae-ei?enoaieo aeaea?ae
aeeth/a? 156 iaeiaioaaiue.

INIIAIEE CI?NO ?IAIOE

O ANOOI? aeaii iaa?oiooaaiiy aeooaeueiino? ?icaeyiooeo a aeena?oaoe??
i?iaeai, noi?ioeueiaai? iaoa ? iniiai? caaea/? aeine?aeaeaiiy,
a?aeia?aaeai? iaoeiaa iiaecia, i?aeoe/ia cia/aiiy oa a??ia?aei?noue
io?eiaieo ?acoeueoao?a, iaaaaeai? iniiai? iieiaeaiiy, ui aeiinyoueny ia
caoeno.

O ?ICAe?E? 1 “Aioo??oiueiiieaeoey?i? eieeai? niaeo?e ooea?ai?a N60 ?
N70” [13A, 17A] cai?iiiiiaaia eieeaia iiaeaeue c i?i?iaeueiei /eneii
ia?aiao??a (/ioe?e iacaeaaei? neeia? noae?), a iaaeao yei? aia?oa
i?iaaaeaii aeaoaeueia oai?aoe/ia aeine?aeaeaiiy aeeiai?/iiai aoaeoo
ssia-Oaeea?a o iieaeoe? N60: ?ic?aoiaai? yi-oae-ea??anuee? aeaoi?iaoe??
oa ?icuaieaiiy aeoeaieo yi-oaeea??anueeeo iiae ooea?aio, i?iaiae?ciaaia
eiai caeeoeiaa neiao??y. Oey eieeaia iiaeaeue ia?aa??aia ia ?ic?a-ooieao
/anoio ? oi?i aioo??oiueiiieaeoey?ieo eieeaaiue ?cieueiaaieo iieaeoe N60
? N70.

.

.

Ia ?en.1.1 (a) ? (a) iieacai? no?oeoo?a ooea?ai?a N60 ? N70 oa
?icoaooaaiiy ?o inae neiao???.

Eieeai? i?aaenoaaeaiiy aeey ?cieueiaaieo iieaeoe N60 ? N70 iathoue oaeee
aeaeyae:

AI(N60)=2Ag + 4F1g + 4F2g + 6Gg + 8Hg + Au + 5F1u + 5F2u + 6Gu +
7Hu. (1.1)

. (1.2)

Aeei?enoiaoth/e ?aeeiee i?aeo?ae uiaei ?ica’ycaiiy aeeiai?/ii? caaea/?
aeey oo-ea?ai?a N60 ? N70, ?o aioo??oiueiiieaeoey?iee niaeo? aoa
?ic?aoiaaiee a iaaeao eieeaii? iiaeae?, yea a?aoiaoaaea eeoa /ioe?e
iacaeaaei? neeia? noae? i?e aecia/aii? iioaioe?aeueii? aia?a?? oeeo
iieaeoe

, (1.3)

aea ki (i=1,2,3,4) – neeia? noae?, ye? oa?aeoa?ecothoue a?aeiinio ci?io
a?aenoai? i?ae aoiiaie aoaeaoeth o i?aaeeueieo i’yoe- (k1) ?
oanoeeooieeao (k2), a oaeiae ci?io aaee/eie eooa o i?aaeeueieo i’yoe-
(k3) ? oanoeeooieeao (k4). ?o /eneia? cia/aiiy iaaaaeai? o Oaae.1.1.

?ic?aoiaai? cia/aiiy /anoio eieeaaiue aeey ?cieueiaaieo iieaeoe N60 ?
N70 eaaeaoue o oaeeo ?ioa?aaeao (i?e T>HON).

1. Noaaeiaei A.E. [8] aoa cai?iiiiiaaiee iaoai?ci ni?i-oiiiiiiai
ca’yceo, yeee a?oioo?oueny ia oiio, ui aiane?aeie ai?cio?ii??
i?aeiieaeoey?ieo aca?iiae?e o iieaeoey?ieo e?enoaeao o?aineyoe?eiee ?oo
oeaio??a ian iieaeoe noi?iaiaeaeo?oueny ci?iith i???ioaoe?? iieaeoey?ieo
inae, oiaoi ia? i?noea ca’ycie iinooiaeueieo ? iaa?oaeueieo ?oo?a
iieaeoee (CII-iaoai?ci). Oaeei /eiii, aeieea? aca?iiae?y ni?iiai?
i?aenenoaie c aeonoe/iith oaeeath ? noa? iiaeeeaith ia?aaea/a aia?a??
a?ae ni?iiai? nenoaie aei a?aoee ? iaaiaee. Oey aca?iiae?y iieno?oueny
aai?eueoii?aiii, yeee ia? aeaeyae

, (4.2)

– iane?i/aiii iaeee eoo iiai?ioo iieaeoee iaaeiei (-? aieiaii? a?n?
?ia?oe??.

aecia/a?oueny, acaaae? eaaeo/e, ia eeoa a?aoeith e?enoaea-iao?eoe?,
aea ? aeanoeainoyie o?eieaoii caoaeaeaii? iieaeoee. Iaeiae, yeui /anoioe
ia?aoiae?a i?ae ni?iiaeie i?ae??aiyie cia/ii iaio? aeaaa?anueei?
/anoioe, oi aieeaii o?eieaoii caoaeaeaii? iieaeoee ia eieeaaiiy a?aoee
iiaeia ciaoooaaoe ? iieeanoe:

(4.3)

– iia?aoi? ia?iaeaeaiiy oiiiia j-? aeonoe/ii? a?oee, (fj – /anoioa
eieeaaiiy, yea aecia/a?oueny e?i?eiei caeiiii aeenia?n??.

,0,1) oioicaoaeaeaii? iieaeoee o ooea?eo?:

(4.4)

. (4.5)

Ooo ( – eoo i?ae aaeoi?ii ?iaeoeoe?? iaai?oiiai iiey A ? iieaeoey?iith
a?nnth x, g – oaeoi? a?eueiiai aeaeo?iia.

Cia/aiiy eiinoaioe ni?i-oiiiiiiai ca’yceo a aoei io?eiaii c aiae?co
??aiyiue aeeiai?ee a?aoee o aeiaaioaeeueiaiio iaaeeaeaii? (f(0), eiee
CII ?oo?a iieaeoee iiaea aooe a?aoiaaiee ca oai???th cao?aiue (aeea.
Aeiaeaoie A). *eneia? ?ic?aooiee cana?ae/eee: a=2.98(102 c-1 Te-3 (o
aeiaaeeo ooea?aio N60) ? a=1.73(102 c-1Te-3 (o aeiaaeeo ooea?aio N70).

2. Aiae?a?aei A.I. oa I?eeooeueeei TH.?. [9] aoa cai?iiiiiaaiee
iaoai?ci ni?i-oiiiiii? aca?iiae??, iaoiiaeaiee ca’yceii iinooiaeueieo
?oo?a iieaeoee ? aioo??oiueiiieaeoey?ieo eieeaaiue ?? yaea?
(CIAE-iaoai?ci), ye? ci?iththoue ?iciiae?e aeaeo?iiii? aonoeie ii
iieaeoe? ?, a?aeiia?aeii, iiaeoeththoue aia?a?th oiiei? no?oeoo?e.
Iniaeeai aeooaeueiei oeae iaoai?ci iiaea aeyaeoeny o aeiaaeeo
aeine?aeaeaiiy ?aeaenaoe?eieo i?ioean?a o ooea?eo? N60, ine?eueee
ci?uaiiy yaea? o o?eieaoii oioicaoaeaeai?e iieaeoe? N60 oaeiae
a?aeaoaathoueny ca ?aooiie aeeiai?/iiai aoaeoo ssia-Oaeea?a.

Ni?i-aai?eueoii?ai caaea/? ia? oaeee aeaeyae:

(4.6)

a iie? aeonoe/ii? oaee? iieno?oueny oi?ioeith

(4.7)

aea M – iana yae?a aoiia aoaeaoeth o iieaeoe?.

?icaeyaeath/e iia?aoi? aca?iiae?? H(CIAE) (4.6) ye cao?aiiy, aoee
?ic?aoiaai? eiia??iino? ia?aoiae?a i?ae ni?iiaeie o?eieaoieie
i?ae??aiyie oioicaoaeaeaii? iieaeoee o ooea?eo?:

(4.8)

(4.9)

=3.78 n-1Oe-5 (aeey iieaeoee N70).

. C oeueiai aeieeaa? aaaeeeaee aeniiaie i?i iiaeeea?noue aeine?aeaeaiiy
oeeo iaoai?ci?a naeaeoeaiei /eiii o ??cieo iaeanoyo iaai?oiiai iiey.

(aeea. Aeiaeaoie

Oaae.4.1

(a c-1) o OCN ooea?eoo N60 aeey ??cieo oaiia?aoo? ? iaai?oieo iie?a
(B((z, z((C2), io?eiai? a iaaeao CII- ? CIAE-iaoai?ci?a.

I?ei?oea. O aeoaeeao iaaaaeai? cia/aiiy eiia??iinoae NA? c o?aooaaiiyi
aieeao aeeiai?/iiai aoaeoo ssia-Oaeea?a o iieaeoe? N60.

eiia??iino? NA? B, Te

T, K

4.2 10 15 20

7.36(102

1.66(103

2.46(103

3.26(103

0.3

2.94

(1.41(101)

6.62

(3.17(101)

9.80

(4.69(101)

1.30(101

(6.22(101)

1.01(104

2.02(104

2.90(104

3.79(104

1

4.47(102

(1.88(103)

8.95(102

(3.76(103)

1.29(103

(5.42(103)

1.68(103

(7.06(103)

6.21(105

8.06(105

1.01(106

1.22(106

5

6.88(105

(1.65(106)

8.93(105

(2.14(106)

1.11(106

(2.66(106)

1.35(106

(3.24(106)

(B2.

(aeea. Oaae.4.1).

I?e aeine?aeaeaii? ni?iiai? ?aeaenaoe?? o c?aceao ii?ioeiaeaeiiai
ooea?eoo N60 [13] a ?ioa?aae? oaiia?aoo? O=(1.7-15) E oa ?iaeoeoe??
iaai?oiiai iiey A=0.3 Oe aenia?eiaioaeueii niinoa??aaee oaeo
oaiia?aoo?io caeaaei?noue /ano NA?: O1=((1+(2T2.5)-1 ((1 ? (2 – iino?ei?
aaee/eie). Oey caeaaei?noue ? aiiiaeueiith c oi/ee ci?o a?aeiieo
?aeaenaoe?eieo iaoai?ci?a. Iaeiae, ?? aaea?oueny iiynieoe a iaaeao
CII-iaoai?cio ni?i-oiiiiii? aca?iiae?? c o?aooaaiiyi ?aiai?anueeeo
aeaioiiiiieo i?ioean?a.

Aai?eueoii?ai caaea/? ia? oaeee aeaeyae:

. (4.10)

?icaeyaeath/e iia?aoi? aca?iiae?? H(CII) (4.10) ye cao?aiiy, aoee
?ic?aoiaai? eiia??iino? ia?aoiae?a i?ae ni?iiaeie o?eieaoieie
i?ae??aiyie oioicaoaeaeaii? iieaeoee o ooea?eo? N60

(4.11)

(4.12)

aea eiinoaioa ni?i-oiiiiii? aca?iiae?? b=1.28(10-6 c-1 K-7 ?

(4.13)

. Ioaea, oe? oeie ?aeaenaoe?eieo i?ioean?a iiaeooue aooe aeine?aeaeai?
ie?aii o ??cieo iaeanoyo oaiia?aoo?e.

Oaiia?aoo?i? caeaaeiino? /ano NA? aeey i?yieo iaeiioiiiiieo (e?eaa 1) ?
?aiai?anueeeo aeaioiiiiieo (e?eaa 2) i?ioean?a i?e aaee/ei? iaai?oiiai
iiey A=0.3 Oe oa eiai i???ioaoe?? (=(/2 (B((z) iaaaaeai? ia ?en.4.1. sse
aeaeii, a iaeano? aae??ai? oaiia?aoo?e aeii?iothoue ?aiai?anuee?
i?ioeane, ui aeaco? ia a?eueo aenieo aonoeio aeaioiiiiieo noai?a, i?ae
iaeiioiiiiieo i?e O=(4.2-5) E. C ?inoii oaiia?aoo?e (T>5 K) ii/eiathoue
aeii?ioaaoe i?yi? iaeiioiiiii? i?ioeane. Io?eiai? ?ic?aooieia?
e?ea? 1 ? 2 aeia?a ocaiaeaeothoueny c ?acoeueoaoaie aenia?eiaioo
[13] (e?eaa 3) a ?ioa?aae? oaiia?aoo? O=(4.2-15) E: i?io?eue e?eai? 2
iiaoi?th? e?eao 3 a iaeano? O=(4.2-5) E, a i?io?eue e?eai? 1 – i?e
5

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